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Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy
Du, Juan; Yuan, Wei; Xing, Xin; Miyatake, Tomohiro; Tamiaki, Hitoshi; Kobayashi, Takayoshi; Leng, Yuxin; kobayashi@ils.uec.ac.jp; lengyuxin@mail.siom.ac.cn
2017
发表期刊Chem. Phys. Lett.
卷号683页码:154
摘要By real-time vibrational spectroscopy using 6.8 fs pulses, real-time vibronic coupling in stair-like zinc chlorin aggregates was studied. Besides the observed fast excitonic relaxation, amplitudes of coherent molecular vibrations are found to be linearly dispersed from the resonant peak as a function of their own vibrational frequencies. In addition, the initial phases of the molecular vibrations exhibiting clear pi phase jump have been observed. All these results indicate that coherent vibrations in the artificial chlorosome intermediate energy exchange between the laser fields around the resonant peak and those separated from it by photon energy equal to the vibrational frequencies.
文章类型Article
部门归属强光
DOI10.1016/j.cplett.2017.05.050
资助者100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology ; 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology ; 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology ; 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology
收录类别SCI
资助者100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology ; 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology ; 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology ; 100 Talents Program of Chinese Academy of Sciences (CAS), Strategic Priority Research Program of CAS [XDB1603, 61475169, 61521093, 11127901]; Japan Science and Technology
WOS记录号WOS:000405802200024
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.siom.ac.cn/handle/181231/28718
专题强场激光物理国家重点实验室
通讯作者kobayashi@ils.uec.ac.jp; lengyuxin@mail.siom.ac.cn
作者单位中国科学院上海光学精密机械研究所
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GB/T 7714
Du, Juan,Yuan, Wei,Xing, Xin,et al. Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy[J]. Chem. Phys. Lett.,2017,683:154.
APA Du, Juan.,Yuan, Wei.,Xing, Xin.,Miyatake, Tomohiro.,Tamiaki, Hitoshi.,...&lengyuxin@mail.siom.ac.cn.(2017).Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy.Chem. Phys. Lett.,683,154.
MLA Du, Juan,et al."Spectral modulation observed in artificial photosynthetic complexes by real-time vibrational spectroscopy".Chem. Phys. Lett. 683(2017):154.
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