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Near Infrared Quantum Cutting Luminescence of Er3+/Tm3+ Ion Pairs in a Telluride Glass
Chen, Xiaobo; Li, Song; Hu, Lili; Wang, Kezhi; Zhao, Guoying; He, Lizhu; Liu, Jinying; Yu, Chunlei; Tao, Jingfu; Lin, Wei; Yang, Guojian; Salamo, Gregory J.; chen78xb@sina.com
2017
Source PublicationSci Rep
Volume7
AbstractThe multiphoton near-infrared, quantum cutting luminescence in Er3+/Tm3+ co-doped telluride glass was studied. We found that the near-infrared 1800-nm luminescence intensity of (A) Er3+(8%) Tm3+(0.5%): telluride glass was approximately 4.4 to 19.5 times larger than that of (B) Tm3+(0.5%): telluride glass, and approximately 5.0 times larger than that of (C) Er3+(0.5%): telluride glass. Additionally, the infrared excitation spectra of the 1800 nm luminescence, as well as the visible excitation spectra of the 522 nm and 652 nm luminescence, of (A) Er3+(8%) Tm3+(0.5%): telluride glass are very similar to those of Er3+ ions in (C) Er3+(0.5%): telluride glass, with respect to the shapes of their excitation spectral waveforms and peak wavelengths. Moreover, we found that there is a strong spectral overlap and energy transfer between the infrared luminescence of Er3+ donor ions and the infrared absorption of Tm3+ acceptor ions. The efficiency of this energy transfer {I-4(13/2)(Er3+) -> I-4(15/2)(Er3+), H-3(6)(Tm3+) -> F-3(4)(Tm3+)} between the Er3+ and Tm3+ ions is approximately 69.8%. Therefore, we can conclude that the observed behaviour is an interesting multiphoton, near-infrared, quantum cutting luminescence phenomenon that occurs in novel Er3+-Tm3+ ion pairs. These findings are significant for the development of next-generation environmentally friendly germanium solar cells, and near-to-mid infrared (1.8-2.0 mu m) lasers pumped by GaN light emitting diodes.
SubtypeArticle
Department单元
DOI10.1038/s41598-017-02244-8
Funding OrganizationNational Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01] ; National Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01] ; National Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01] ; National Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01]
Indexed BySCI
Funding OrganizationNational Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01] ; National Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01] ; National Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01] ; National Natural Science Foundation of China [51472028]; Fundamental Research Funds for the Central Universities of China [2017TZ01]
WOS IDWOS:000401406700051
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Cited Times:1[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.siom.ac.cn/handle/181231/28305
Collection高功率激光单元技术研发中心
Corresponding Authorchen78xb@sina.com
Affiliation中国科学院上海光学精密机械研究所
Recommended Citation
GB/T 7714
Chen, Xiaobo,Li, Song,Hu, Lili,et al. Near Infrared Quantum Cutting Luminescence of Er3+/Tm3+ Ion Pairs in a Telluride Glass[J]. Sci Rep,2017,7.
APA Chen, Xiaobo.,Li, Song.,Hu, Lili.,Wang, Kezhi.,Zhao, Guoying.,...&chen78xb@sina.com.(2017).Near Infrared Quantum Cutting Luminescence of Er3+/Tm3+ Ion Pairs in a Telluride Glass.Sci Rep,7.
MLA Chen, Xiaobo,et al."Near Infrared Quantum Cutting Luminescence of Er3+/Tm3+ Ion Pairs in a Telluride Glass".Sci Rep 7(2017).
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