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Hybrid coordination-network-engineering for bridging cascaded channels to activate long persistent phosphorescence in the second biological window
Qin, Xixi; Li, Yang; Zhang, Ruili; Ren, Jinjun; Gecevicius, Mindaugas; Wu, Yiling; Sharafudeen, Kaniyarakkal; Dong, Guoping; Zhou, Shifeng; Ma, Zhijun; Qiu, Jianrong; msliyang@scut.edu.cn; qjr@scut.edu.cn
2016
发表期刊Sci Rep
卷号6
摘要We present a novel "Top-down" strategy to design the long phosphorescent phosphors in the second biological transparency window via energy transfer. Inherence in this approach to material design involves an ingenious engineering for hybridizing the coordination networks of hosts, tailoring the topochemical configuration of dopants, and bridging a cascaded tunnel for transferring the persistent energy from traps, to sensitizers and then to acceptors. Another significance of this endeavour is to highlight a rational scheme for functionally important hosts and dopants, Cr/Nd co-doped Zn1-xCaxGa2O4 solid solutions. Such solid-solution is employed as an optimized host to take advantage of its characteristic trap site level to establish an electron reservoir and network parameters for the precipitation of activators Nd3+ and Cr3+. The results reveal that the strategy employed here has the great potential, as well as opens new opportunities for future new-wavelength, NIR phosphorescent phosphors fabrication with many potential multifunctional bio-imaging applications.
文章类型Article
部门归属材料
DOI10.1038/srep20275
资助者National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2 ; National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2 ; National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2 ; National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2
收录类别SCI
资助者National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2 ; National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2 ; National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2 ; National Natural Science Foundation of China [51132004, 51072754, 51472091, 61475174]; Guangdong Natural Science Foundation [S2011030001349, 2014A030310444]; National Basic Research Program of China [2011CB808100]; China Postdoctoral Science Foundation [2
WOS记录号WOS:000369270100002
引用统计
被引频次:6[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.siom.ac.cn/handle/181231/28102
专题中科院强激光材料重点实验室
通讯作者msliyang@scut.edu.cn; qjr@scut.edu.cn
作者单位中国科学院上海光学精密机械研究所
推荐引用方式
GB/T 7714
Qin, Xixi,Li, Yang,Zhang, Ruili,et al. Hybrid coordination-network-engineering for bridging cascaded channels to activate long persistent phosphorescence in the second biological window[J]. Sci Rep,2016,6.
APA Qin, Xixi.,Li, Yang.,Zhang, Ruili.,Ren, Jinjun.,Gecevicius, Mindaugas.,...&qjr@scut.edu.cn.(2016).Hybrid coordination-network-engineering for bridging cascaded channels to activate long persistent phosphorescence in the second biological window.Sci Rep,6.
MLA Qin, Xixi,et al."Hybrid coordination-network-engineering for bridging cascaded channels to activate long persistent phosphorescence in the second biological window".Sci Rep 6(2016).
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