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Generic synthesis and versatile applications of molecularly organic-inorganic hybrid mesoporous organosilica nanoparticles with asymmetric Janus topologies and structures
Tao, Guiju; Bai, Zhengyuan; Chen, Yu; Yao, Heliang; Wu, Meiying; Huang, Ping; Yu, Luodan; Zhang, Jiamin; Dai, Chen; Zhang, Long; chenyu@mail.sic.ac.cn; lzhang@siom.ac.cn
2017
Source PublicationNano Res.
Volume10Issue:11Pages:3790
AbstractPrecise control over the morphology, nanostructure, composition, and particle size of molecularly organic-inorganic hybrid mesoporous organosilica nanoparticles (MONs) still remains a major challenge, which severely restricts their broad applications. In this work, an efficient bridged organic group-determined growth strategy has been proposed for the facile synthesis of highly dispersed and uniform MONs with multifarious Janus morphologies, nanostructures, organic-inorganic hybrid compositions, and particle sizes, which can be easily controlled simply by varying the bridged organic groups and the concentration of bis-silylated organosilica precursors used in the synthesis. In addition, the formation mechanism of Janus MONs determined by the bridged organic group has been discussed. Based on the specific structures, compositions, and asymmetric morphologies, all the synthesized Janus MONs with hollow structures (JHMONs) demonstrate excellent performances in nanomedicine as desirable drug carriers with high drug-loading efficiencies/capacities, pH-responsive drug releasing, and enhanced therapeutic efficiencies, as attractive contrastenhanced contrast agents for ultrasound imaging, and as excellent bilirubin adsorbents with noticeably high adsorption capacities and high blood compatibilities. The developed versatile synthetic strategy and the obtained JHMONs are extremely important in the development and applications of MONs, particularly in the areas of nanoscience and nanotechnology.
SubtypeArticle
Department材料
DOI10.1007/s12274-017-1592-5
Funding OrganizationNational Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents ; National Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents ; National Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents ; National Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents
Indexed BySCI
Funding OrganizationNational Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents ; National Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents ; National Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents ; National Key Research and Development Program of China [2016YFA0203700]; Shanghai Natural Science Foundation [16ZR1440300]; National Natural Science Foundation of China [61275208, 51302293, 51672303]; Shanghai Rising-Star Program [14QA1404100]; Youth Innovation Promotion Association of the Chinese Academy of Sciences [2013169]; Development Fund for Shanghai Talents
WOS IDWOS:000413100400017
Citation statistics
Document Type期刊论文
Identifierhttp://ir.siom.ac.cn/handle/181231/28086
Collection中科院强激光材料重点实验室
Corresponding Authorchenyu@mail.sic.ac.cn; lzhang@siom.ac.cn
Affiliation中国科学院上海光学精密机械研究所
Recommended Citation
GB/T 7714
Tao, Guiju,Bai, Zhengyuan,Chen, Yu,et al. Generic synthesis and versatile applications of molecularly organic-inorganic hybrid mesoporous organosilica nanoparticles with asymmetric Janus topologies and structures[J]. Nano Res.,2017,10(11):3790.
APA Tao, Guiju.,Bai, Zhengyuan.,Chen, Yu.,Yao, Heliang.,Wu, Meiying.,...&lzhang@siom.ac.cn.(2017).Generic synthesis and versatile applications of molecularly organic-inorganic hybrid mesoporous organosilica nanoparticles with asymmetric Janus topologies and structures.Nano Res.,10(11),3790.
MLA Tao, Guiju,et al."Generic synthesis and versatile applications of molecularly organic-inorganic hybrid mesoporous organosilica nanoparticles with asymmetric Janus topologies and structures".Nano Res. 10.11(2017):3790.
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