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Functionalization of reduced graphene oxide with axially-coordinated metal-porphyrins: facile syntheses and temporally-dependent nonlinear optical properties
Wang, Aijian; Song, Jingbao; Jia, Ding; Yu, Wang; Long, Lingliang; Song, Yinglin; Cifuentes, Marie P.; Humphrey, Mark G.; Zhang, Long; Shao, Jianda; Zhang, Chi; chizhang@jiangnan.edu.cn
2016
Source PublicationInorg. Chem. Front.
Volume3Issue:2Pages:296
AbstractReduced graphene oxide-tin porphyrin (RGO-SnTPP) nanohybrids with good dispersibility have been prepared by two covalent functionalization approaches. The microscopic structure and morphology of the RGO-SnTPP nanohybrids were characterized by various spectroscopic techniques including Fourier transform infrared spectroscopy, Raman spectroscopy, transmission electron microscopy, thermogravimetric analysis and X-ray photoelectron spectroscopy. Ground-state absorption and steady-state fluorescence studies indicate considerable pi-pi interactions and effective photo-induced electron and/or energy transfer from the porphyrin moieties to the RGO. Their nonlinear optical properties were investigated using the Z-scan technique at 532 nm with both picosecond and nanosecond laser pulses. The RGO-SnTPP hybrids were found to exhibit large nonlinear optical responses due to a combination of mechanisms, while significant differences in their nonlinear optical responses were observed, highlighting the influence on photophysical properties of the degree of functionalization and the synthetic approach employed.
SubtypeArticle
Department材料
DOI10.1039/c5qi00209e
Funding OrganizationNational Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T ; National Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T ; National Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T ; National Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T
Indexed BySCI
Funding OrganizationNational Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T ; National Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T ; National Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T ; National Natural Science Foundation of China [51432006, 50925207, 51172100]; Ministry of Science and Technology of China for the International Science Linkages Program [2011DFG52970]; Ministry of Education of China for the Changjiang Innovation Research T
WOS IDWOS:000371162200012
Citation statistics
Document Type期刊论文
Identifierhttp://ir.siom.ac.cn/handle/181231/28085
Collection中科院强激光材料重点实验室
Corresponding Authorchizhang@jiangnan.edu.cn
Affiliation中国科学院上海光学精密机械研究所
Recommended Citation
GB/T 7714
Wang, Aijian,Song, Jingbao,Jia, Ding,et al. Functionalization of reduced graphene oxide with axially-coordinated metal-porphyrins: facile syntheses and temporally-dependent nonlinear optical properties[J]. Inorg. Chem. Front.,2016,3(2):296.
APA Wang, Aijian.,Song, Jingbao.,Jia, Ding.,Yu, Wang.,Long, Lingliang.,...&chizhang@jiangnan.edu.cn.(2016).Functionalization of reduced graphene oxide with axially-coordinated metal-porphyrins: facile syntheses and temporally-dependent nonlinear optical properties.Inorg. Chem. Front.,3(2),296.
MLA Wang, Aijian,et al."Functionalization of reduced graphene oxide with axially-coordinated metal-porphyrins: facile syntheses and temporally-dependent nonlinear optical properties".Inorg. Chem. Front. 3.2(2016):296.
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