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Coherent control of the dissociation probability of H-2(+) in omega-3 omega two-color fields
Xu, Han; Hu, Hongtao; Tong, Xiao-Min; Liu, Peng; Li, Ruxin; Sang, Robert T.; Litvinyuk, Igor V.; peng@siom.ac.cn; ruxinli@mail.shcnc.ac.cn
2016
Source PublicationPhys. Rev. A
Volume93Issue:6
AbstractWe demonstrate that the coherent control of unimolecular reactions by using a waveform-controlled laser fields can lead to a strong modulation on the yield of the reaction. By using a synthesized omega (1800-nm) and 3 omega (600-nm) two-color laser field, the probability of photodissociation of H-2(+) can be strongly modulated by varying the relative phase between the two colors. The dissociation probability maximizes at different relative phases for protons with different kinetic energy, and such energy dependence can also be qualitatively reproduced by our simulation. We attribute the observed dissociation probability modulation to the interference between two different dissociation pathways which start from the same electronic states and end with the same kinetic energy.
SubtypeArticle
Department强光
DOI10.1103/PhysRevA.93.063416
Funding OrganizationAustralian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628]; ; Australian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628]; ; Australian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628]; ; Australian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628];
Indexed BySCI
Funding OrganizationAustralian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628]; ; Australian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628]; ; Australian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628]; ; Australian Research Council (ARC) Discovery Project [DP110101894]; ARC Centre for Coherent X-Ray Science [CE0561787]; National Science Foundation of China [11274326, 61221064, 11134010, 11127901]; ARC Discovery Early Career Researcher Award [DE130101628];
WOS IDWOS:000378048900005
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Document Type期刊论文
Identifierhttp://ir.siom.ac.cn/handle/181231/27572
Collection强场激光物理国家重点实验室
Corresponding Authorpeng@siom.ac.cn; ruxinli@mail.shcnc.ac.cn
Affiliation中国科学院上海光学精密机械研究所
Recommended Citation
GB/T 7714
Xu, Han,Hu, Hongtao,Tong, Xiao-Min,et al. Coherent control of the dissociation probability of H-2(+) in omega-3 omega two-color fields[J]. Phys. Rev. A,2016,93(6).
APA Xu, Han.,Hu, Hongtao.,Tong, Xiao-Min.,Liu, Peng.,Li, Ruxin.,...&ruxinli@mail.shcnc.ac.cn.(2016).Coherent control of the dissociation probability of H-2(+) in omega-3 omega two-color fields.Phys. Rev. A,93(6).
MLA Xu, Han,et al."Coherent control of the dissociation probability of H-2(+) in omega-3 omega two-color fields".Phys. Rev. A 93.6(2016).
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